Experimental techniques for chemical bonding measurements have been confined to homogeneous crystalline materials. Over the last two decades, quantitative convergent beam electron diffraction (QCBED) has emerged as the most accurate and precise technique for such measurements [1 - 3] and, with recent advances, it has been suggested that QCBED may be the only way to measure bonding in nano-composite materials [4].
In this work, we present the first attempts to measure bonding in an inhomogeneous crystalline material. We apply the multislice formalism [5] for electron scattering in our approach to QCBED (which requires the material being characterised to be sliced into layers) to examine the structures of the plate-like strengthening precipitates of the theta' and theta" phases in an aluminium-copper alloy, at atomic and electronic resolution.